Bernard Baxley / Carmichael / Chief / Dr. Morell Mackenzie / Mr. Lamb / Old seaman / Wethers / Wilf
Andrew Undershaft / Archbishop / Burghley / Butler / Cardinal Inquisitor / Grandpa / Jason / Joshua / Julius Caesar / Lord Caversham / Mr. Wemmick / Rev. Robert / Sir Patrick Cullen / The Clairvoyant / The Professor / Zvierkov / matchseller (segment "A Slight Ache")
Police officer / Dr. Curtis Connor / Dr. Smartyr / ...
The Leader / Khanga Khan (voice)
Zemo / Radioactive Man / Additional Voices (voice)
Lord Caversham / Rev. Robert / The Professor / ...
Del Prado / Ghat
Old seaman / Wilf / Chief / ...
Mr. Justice Byrne
Frederick Dove / Mr. Kosak / Dr. Stewart / ...
Archangel / Alex
Variety / Don Bernal / Triptolemus / ...
Mr. Thomson / Lawrence
T. Gilly Fenwick | T.G. Fenwick
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